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|''The Nun's Story''|| || Õde Luke (Gabrielle van der Mal) ||
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| 1960 || ''[[The Unforgiven'' (1960 film)|The Unforgiven]]''| || Rachel Zachary ||
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| rowspan="2"|1961 || ''[[Breakfast at Tiffany's (film)|Breakfast at Tiffany's]]'' || || Holly Golightly || Nominated — [[Academy Award for Best Actress]]
|-
|''[[The Children's Hour'' (1961 film)|The Children's Hour]]''| || Karen Wright ||
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| 1963 || ''[[Charade (film)|Charade]]'' || || Regina "Reggie" Lampert ||[[BAFTA Award for Best Actress in a Leading Role]]<br /> Nominated — [[Golden Globe Award for Best Actress – Motion Picture Musical or Comedy]]
|-
| rowspan="2"|1964 || ''[[Paris When It Sizzles]]'' || || Gabrielle Simpson ||
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|''[[My Fair Lady'' (film)|My| Fair''[[Minu Ladyveetlev leedi]]'' || Eliza Doolittle || Nominated — [[Golden Globe Award for Best Actress – Motion Picture Musical or Comedy]]
|-
| 1966 || ''[[How to Steal a Million]]'' || || Nicole Bonnet ||
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| rowspan="2"|1967 || ''[[Two for the Road (1967 film)|Two for the Road]]'' || || Joanna Wallace || Nominated — [[Golden Globe Award for Best Actress – Motion Picture Musical or Comedy]]
|-
|''Wait Until Dark'' || || Susy Hendrix ||
|''[[Wait Until Dark (film)|Wait Until Dark]]'' || Susy Hendrix || Nominated — [[Academy Award for Best Actress]]<br />Nominated — [[Golden Globe Award for Best Actress – Motion Picture Drama]]
|-
| 1976 || ''[[Robin and Marian]]'' || [[Maid Marian|Lady| Marian]] ||
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| 1979 || ''[[Bloodline (film)|Bloodline]]'' || || Elizabeth Roffe || Her only R-rated film
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| 1981 || ''[[They All Laughed]]'' || || Angela Niotes ||
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| 1989 || ''[[Always'' (1989 film)|Always]]''| || Hap ||
|}
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